Thanks for the warning, Ranch. I wondered how hard it would be to get it perfectly round with that kind of equipment; the guy in the article made it sound simple. I found all the things he did to be very interesting, and quite honestly, I enjoy working with my guns myself. I've done a good bit of amateur gunsmithing, but am certainly a newbie with the single actions. I do think I could buy the tool from Brownells and do a good job with it, but it would probably be cheaper to send the cylinder somewhere to a gunsmith.
And I have by no means already decided to do anything to it; will certainly take your advice and shoot it a lot first. However, there is no denying that there is a big difference in the dimensions of this gun and my SAA. I'd sure like to have loads that work equally well in each gun. All the loads I've shot in the Ruger were based on Unique. I tried Blue Dot in the SAA, but got better results with Unique. I'm gonna load up some ammo and set up sand bags and see what it will do as soon as I have time.
edit: Tacklebury, thanks for the info!
Thanks again for all the help.