I am sure there are a lot of people here that know more about bullet casting than I do, but I will give you my opinion. You need to know the hardness of the material you have, the hardness of the material you want to add, and the speed at which you want to achive with your bullets.
The lead from the jacketed bullets will probably be a lot softer than the lead from the cast bullets. So if you collected a lot more jacketed bullets your mixture will be softer than if you collected more cast bullets.
It kind of depends what you want to do with the bullets. If your just plinking it doesn't matter, just check your barrel for leading and back off on you loads if it's apparent. If your hunting you want the bullets hard enough to give good velocity, but not so hard that they don't mushroom, or fragment. If you want top velocity target loads than the harder the better.
Midway has the Lee hardness tester on sale this month. I havn't used it myself but plan on giving one a try. You also might want to go to Beartooth bullets and check out their forums, they have a lot of stuff on cast bullets.